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Measurements of High-Field THz Induced Photocurrents in Semiconductors. Michael Wiczer University of Illinois – Urbana-Champaign Mentor: Prof. Aaron Lindenberg. THz Radiation. 1 THz ~ 33 cm -1 ~ .3 mm ~ 4 meV Few mainstream applications until recently Absorption measures free electrons
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Measurements of High-Field THz Induced Photocurrents in Semiconductors Michael Wiczer University of Illinois – Urbana-Champaign Mentor: Prof. Aaron Lindenberg
THz Radiation • 1 THz ~ 33 cm-1 ~ .3 mm ~ 4 meV • Few mainstream applications until recently • Absorption measures free electrons • Time resolved spectroscopists and condensed matter physicists have used THz as a probe of free electrons in time-resolved studies for some time 1Fedrici et al, IEEE Spectrum, 44, 47
THz Radiation • Half-cycle pulse • Watch a test particle in short times • Quasi-DC field 25 fs 300fs
THz Generation Experiment Space Ti:Sapph Oscillator (800 nm) 25 fs pulses @ 10 nJ 100 MHz rep. rate Regen. Amplifier (800 nm) Chirped Pulse Amplification 50 fs pulses @ 1 mJ 1 KHz rep. rate Frequency Doubling BBO crystal Plasma in air (non-linear optical medium) THz propagation (collimated and focused)
THz Generation Propagation Direction
InSb Experiment • Effective mass: 0.014 me • Band Gap: 0.17 eV (Si band gap = 1.12 eV) • 1 THz photon: 4 meV<<170 meV X Z
InSb Experiment • Measure transmission as beam focuses • Total incident intensity constant • Transmission drops!!! • Generate free carriers?
Avalanche Multiplication • Lose one band-gap of kinetic energy each collision • Require field to be present for longer than collision timescale • Electron energy drops below ionization threshold after only a few collisions w/o field E Field = conduction band e- = valence band e-
Photoconductive Antenna Silver paint electrodes on surface of InSb • Measure currents • Ultrafast detector! • If electron lifetimes are much longer than pulse width, current indicates free carriers generated during pulse duration. Gap ~500 μm
Photoconductive Antenna Current Amplifier 1 pA/V ~4s output time const Lock-in amplifier Time const. 100s Optical Shutter Modulate beam at .2 Hz
Why So Much Amplification? • Measuring very small currents • Considerable noise
Current Measurement • Transverse scan looks like a beam • Suggest THz induced current X Z
Current Measurement • Initial longitudinal scan much broader than transmission z-scan • Scattered IR light induced broadening? • Requires repetition X Z
Conclusions • Non-linear effect has been observed and characterized with bolometer • Tentative measurements of photocurrents have been recorded • We believe to have a prototype ultrafast photodetector
Further Investigation • Repeat current measurement with current induced by scattered IR light eliminated • Apply a voltage bias to isolate free-carrier measurement • Complete our physical picture of this process • Fit data to impact ionization model (or some other mechanism) • Further develop ultrafast detector
Acknowledgements • Lindenberg Group • DOE • SLAC • SULI