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Ground-based logistics / results on Djougou (Bénin). Objectives : obtain measurements of physical, chemical and radiative properties of mixed aerosol (dust & biomass burning) during the dry season in WA study the modification of the radiative budget by aerosols at local scale.
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Ground-based logistics / results on Djougou (Bénin) Objectives : • obtain measurements of physical, chemical and radiative properties of mixed aerosol (dust & biomass burning) during the dry season in WA • study the modification of the radiative budget by aerosols at local scale
What do we measure during SOP_0 / aerosol microphysical properties • aerosol number size distribution (0.05 – 0.5 µm) from SMPS • aerosol number size distribution (0.5 – 10 µm) from GRIMM • particle number concentration aerosol radiative properties from Mie theory (number size distribution and refractive index from chemical composition) derived properties optical closure with ground-based radiative measurements • aerosol mass size distribution for major ions, BC and • OC from impactor Dekati (13 stages)
What do we measure during SOP_0 / aerosol radiative properties • light absorption coefficient (σap) from MAGEE aethalometer (at 7) • at the surface derived properties aerosol single scattering albedo (at 520nm) at the surface • light scattering coefficient (σsp) from ECOTECH nephelometer • (at 520nm) at the surface PHOTON / LOA • aerosol optical depth (440, 670, 870 and 1020nm) • aerosol volume size distribution (0.05 < r < 10 µm) for total atmospheric • column (Dubovik et al., 2002) • aerosol single scattering albedo and asymmetry parameter (at 4 ) for • the total atmospheric column (Dubovik et al., 2002) derived properties vertical profiles of aerosol extinction coefficient & angström exponent (Coll. SA) • vertical profiles of aerosol backscattering coefficients (Coll. SA)
Aerosol optical depth & aerosol size distribution of mixed aerosols on Djougou SOP_0 AOD_scattering AOD_absorption AOD • strong AOD during SOP_0 with AOD 0.9 at 440nm • extinction mostly due to scattering but also by absorption of solar radiations ( 5-20 %) Aerosol optical depth at 440nm • bimodal size distribution with a fine ( 0.1 µm) and a coarse mode ( 1-10µm) • mixing between dust (dominant) and BB confirmation with chemical measurements • comparison with retrievals on Niamey ?? • comparison with ground-based measurements SOP_0 Radius (µm)
Aerosol single scattering albedo of mixed aerosols on Djougou SOP_0 strong absorbing mixed aerosols for the total atmospheric column with SSA 0.84 0.04 at 440nm Aerosol single scattering albedo (440 nm) strong absorbing mixed aerosols at the surface with SSA 0.87 at 520nm some differences appear between SSA estimated at the surface and those inverted for the atmospheric column Lidar measurements nephelometer & aethalometer Aerosol single scattering albedo (520 nm) SOP_0
Asymmetry factor of mixed aerosols on Djougou g is higher on Djougou gSOP_O 0.68 compared to other campaigns, due to the presence of dust aerosols.
Direct radiative forcing of mixed aerosols at local scale / first results • future works to improve the estimation of the local direct radiative effect : • use pyranometer measurements for comparison with downwards fluxes simulated • with radiative transfer model • use satellite sensor (MODIS) for comparison with upwards radiance simulated with • radiative transfer model • use Lidar measurements for estimating the vertical profiles of aerosol extinction • use RH, O3 and T° profiles estimated from balloons for upper atmosphere AOD SSA Wavelenght (nm) strong heating of the aerosol layer Direct radiative forcing (W.m-2) asymmetry factor strong cooling at the surface Wavelenght (nm)
Vertical profiles used in radiative transfer modelling AOD 0.75 (550nm)
Fluxes measurements Meteorological conditions NO emissions At ground level The other parameters… NOx-O3- CO