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SWAPS 2014– Geneva, June 12th, 2014. Double Beta Decay and scintillating bolometers. Andrea Giuliani CNRS/IN2P3/CSNSM Orsay , France. Outline. Introduction to Double Beta Decay Experimental challenges Factors driving isotope and technology choice.
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SWAPS 2014– Geneva, June 12th, 2014 • Double Beta Decay • and scintillating bolometers Andrea Giuliani CNRS/IN2P3/CSNSM Orsay, France Outline • Introduction to Double Beta Decay • Experimental challenges • Factorsdriving isotope and technologychoice • A promisingtechnology: scintillatingbolometers • LUCIFER • LUMINEU • AMoRE
2n Double Beta Decay allowed by the Standard Model already observed – t1018 – 1021 y NeutrinolessDouble Beta Decay (0n-DBD) never observed t > 1025 y (A,Z) (A,Z+2) + 2e- Processe would imply new physics beyond the Standard Model (A,Z) (A,Z+2) + 2e- + 2ne violation of total lepton number conservation • Decay modes for Double Beta Decay Why is neutrinoless Double Beta Decay important • Majorana nature of neutrino (irrespectively of the mechanism) • See-saw mechanism naturalness of small neutrino masses • Leptogenesis and matter-antimatter asymmetry in the Universe
Phase space Nuclear matrix elements Effective Majorana mass neutrinoless Double Beta Decay rate 1/t = G(Q,Z) |Mnucl|2Mbb2 what the experimentalists try to measure parameter containing the physics: Effective Majorana mass what the nuclear theorists try to calculate • The mass mechanism How 0n-DBDis connected to neutrino mixing matrix and masses in case of process induced by light n exchange (mass mechanism) Mbb= ||Ue1 |2M1 + eia1 | Ue2 |2M2 + eia2 |Ue3 |2M3 |
direct inverted Neutrino mass hierarchy Mbb[eV] KlapdorKrivosheinaModern PhysicsLettersA 21, No. 20 (2006) 1547 Lightest neutrino mass [eV]
Three challenges for 0n-DBD search 100-1000 counts/y/ton Mbb[eV] KlapdorKrivosheinaModern PhysicsLettersA 21, No. 20 (2006) 1547 Klapdor’s claim Currentgeneration GEN1 10-100 kg 0.5-5 counts/y/ton 20 meV Nextgeneration GEN2 0.2-1 ton 0.1-1 counts/y/(100 ton) 1 meV Long termgeneration GEN3 >10 ton Lightest neutrino mass [eV]
Approach the inverted hierarchy region [GEN1] Sensitivity at the level of 1-10 counts / y ton Coverthe inverted hierarchy region [GEN2] Sensitivity at the level of 0.1 -1 counts / y ton Order of magnitude of the target bakground in the Region Of Interest: 1 counts / y ton Background demands
Signal and background sources 100Mo 7.1x1018 y • Natural radioactivity of materials • (source itself, surrounding structures) 136Xe 2.2x1021 y • Neutrons (in particular muon-induced) • Cosmogenic induced activity (long living) d=DE/Q • 2nDouble Beta Decay
Background index and energy resolution DE Take energy resolution [keV] b Take background index [counts/(keV kg y)] DExb Multiply them [counts/(kg y)] DExbxMxT Multiply by detector mass, live time → bkg counts Nlim (DExbxMxT)½ Calculate limit T x Nat/ Nlim Limit: invert, multiply by number of atoms and live time Figure of Merit for the technology Scalability of the technology Isotopic abundance and enrichment b 10-1in « classical » source=detector experiments b 10-2 - 10-3in current source=detector and in classicalexternal-source experiments b 10-4 in future experiments (minimum request to coverinvertedhierarchy)
Factors guiding isotope selection No super-isotope in terms of nuclearmatrixelements Phase space: G(Q,Z) Q5 Qis the crucial factor Background End-point of 222Rn-induced radioactivity NineMagnificent End-point of natural g radioactivity
Factors guiding isotope selection No super-isotope in terms of nuclearmatrixelements Phase space: G(Q,Z) Q5 Qis the crucial factor Background End-point of 222Rn-induced radioactivity NineMagnificent Golden isotopes End-point of natural g radioactivity
Isotope, enrichment and technique 48Ca (CANDLES) 150Nd (SuperNEMO?) 82Se (SuperNEMO baseline) Scintillating bolometers (LUCIFER, LUMINEU, AMoRE) 76Ge (GERDA, MAJORANA) 130Te (CUORE, SNO+) 136Xe (EXO, KamLAND-Zen, NEXT)
Basic structure of a bolometer Cryogenicheatsink (10-20 mK) Alpha surface background Thermal and mechanicallink • Thermometer • Phonon signal • - NTD Ge thermistors • - Transition EdgeSensor • MMC magneticsensor Gamma background Phonons The nuclear energy is measured as a temperature increaseof a single crystal e- DBD event e- DT = E/C Crystal (0.5 – 1 kg) containing the source DT DV Thanks to the thermistor Typical signal sizes: 0.1 mK / MeV, converted to about 0.1-0.5 mV / MeV
CUORE Technique/location: natural 988 TeO2 bolometers at 10-15 mK– LNGS (Italy) A.I. (130Te) = 34% (all the other isotopes have <10%) - evolution of Cuoricino Source: TeO2 – 741 kg with natural tellurium (206 kg of 130Te) - 9.5x1026 nuclides of 130Te Sensitivity (90% cl): 40 – 100 meV (5 years) – approach/touch inverted hierarchy region (GEN1) Timeline: first CUORE tower in 2013 (CUORE-0) – taking data Data taking with full apparatus in 2015 – 18 towers over 19 completed – cryostat proceeds well Detector in the custom refrigerator Structure of the detector Expected background index: b 10-2
CUORE-0 - performance First CUORE towernow operating in the former Cuoricino cryostat Excellent detector and background results DEFWHM 5 keV
CUORE-0 - background Energy-degraded alpha background level
Scintillating bolometers and DBD Bolometric technique (CUORE) Simultaneous detection of heat and light + Full alpha/beta separation Choice one of golden isotopes Q-value > 2615 keV “zero” gamma background “zero” alpha background = zero background at the ≈ 1 ton x year scale Achievable goals: Control internal contamination of the crystals 214Bi(238U – 226Ra) 208Tl (232Th – 228Th) High Q-value b transitions b 10-4 counts/(keV kg y) DE < 10 keV 10 mBq/kg
List of interesting crystals Isotope I. A. [%] Q-value Materials successfully tested as bolometers [keV] in crystalline form 76Ge 7.8 2039Ge 136Xe 8.9 2479NONE 130Te 33.8 2527TeO2 116Cd 7.5 2802 CdWO4, CdMoO4 82Se 9.2 2995 ZnSe 100Mo 9.6 3034 PbMoO4, CaMoO4, SrMoO4, CdMoO4, SrMoO4,ZnMoO4,Li2MoO4, MgMoO4 96Zr 2.8 3350 ZrO2 150Nd 5.6 3367 NONE → many attempts 48Ca 0.187 4270 CaF2, CaMoO4 Seven excellent candidates can be studied with high energy resolution and with the bolometric approach
List of interesting crystals Isotope I. A. [%] Q-value Materials successfully tested as bolometers [keV] in crystalline form 76Ge 7.8 2039Ge 136Xe 8.9 2479NONE 130Te 33.8 2527TeO2 116Cd 7.5 2802 CdWO4, CdMoO4 82Se 9.2 2995 ZnSe 100Mo 9.6 3034 PbMoO4, CaMoO4, SrMoO4, CdMoO4, SrMoO4,ZnMoO4,Li2MoO4, MgMoO4 96Zr 2.8 3350 ZrO2 150Nd 5.6 3367 NONE → many attempts 48Ca 0.187 4270 CaF2, CaMoO4 Compounds in boldface are reasonable / good scintillators Ruled out by lowisotopicabundance and difficultenrichement Four golden candidates (116Cd – 100Mo – 82Se – 48Ca) can be studied as scintillating bolometers
Concept of a scintillating bolometer for double beta decay Auxiliarybolometer for light detection
Experimental situation Intense R&D activity in the framework of threeprojects: LUCIFER (ERC advancedgrant – INFN Italy, Orsay France) ZnSe LUMINEU (funded by ANR - France, Ukraine, Russia, Germany) ZnMoO4 AMoRE (Korea, Russia, Ukraine, China, Germany, Pakistan) CaMoO4 Proof of concept essentiallydemonstratedin all the three cases. At LNGS, positive resultsobtainedalso for CdWO4 and Li2MoO4 In two-yearscale, a 10-kg-isotope experimentis possible for the three cases. GEN1 experimentsapproaching the invertedhierarchy mass region
ZnSe – LUCIFER – crystal production (or even75%)
ZnSe – LUCIFER – single module performance PSD in the heatchannel PSD in the light channel
ZnSe – LUCIFER – Background This and following slides about LUCIFER are from S. Pirro From Majorana to LHC: Workshop on the Origin of Neutrino Mass, Trieste 3 October 2013
ZnSe – LUCIFER – Experiment scheme LNGS CUORE-0 cryostat
ZnSe – LUCIFER – Schedule Delay of about 6 months due to the crystallization issue Adv. High En. Phys. 2013 (2013) 237973
ZnMoO4 – LUMINEU Purification of MoO3 and crystallization Bothperformedat the NikolaevInstute of InorganicChemistry, Novosibirsk, Russia JINST 09 (2014) P06004 Double purification step (1) Sublimation of MoO3 in vacuum (2) Re-crystallizationfromaqueous solution of ammonium molybdate
ZnMoO4 – LUMINEU Purification of MoO3 and crystallization JINST 09 (2014) P06004 Crystallization by low-thermal gradient Czochralski technique Large cylindricalcrystalswith excellent opticalproperties Ø = 5 cm – h = 4 cm – M = 340 g
ZnMoO4 – LUMINEU Preliminary test on a 313 g crystal 313 g crystalgrown at NIIC (Novosibrisk, Russia) Assemblyadapted to EDELWEISS holder structure
ZnMoO4 – LUMINEU Preliminary test on a 313 g crystal
ZnMoO4 – LUMINEU 232Th calibration in the EDELWEISS cryostat (LSM)
ZnMoO4 – LUMINEU Scatter plot light vs. heat Light yield for betas: 1 keV/MeV Alpha quenching factor: 0.15
ZnMoO4 – LUMINEU Alpha/beta discrimination power (gamma-calibratedscale)
ZnMoO4 – LUMINEU Background spectrum (alpha region)
ZnMoO4 – LUMINEU Internal contamination
ZnMoO4 – LUCIFER Tests at LNGS Similarly excellent resultshave been obtained in the framework of LUCIFER at LNGS with a twincrystalcomingfrom the same boule Eur. Phys. J. C 72 (2012) 2142 Withthree detectors with a total mass of 811 g, the two neutrino double beta decayof 100Mohalf life wasmeasuredwith a T1/2 = 7.15 ± 0.37 (stat.) ± 0.66 (syst.) ·1018 y (1. 3 kg day of exposure for 100Mo) NEMO3 results: 7.17 ± 0.01 (stat) ± 0.54 (syst) ·1018 y (with 6.9 kg of 100Mo)
ZnMoO4 – LUMINEU Enrichedcrystals First Zn100MoO4 boule wasgrownfromdeeplypurified100Mo Twosampleswith masses 64 g and 61 gwereproduced The reasonwhycrystals are smallisthat in the first attemptwedecided to use a smallamount of enrichedmaterial in a smallcrucible Irrecoverablelosses of the purification/crystallizationprocesses: < 4 % Production of large mass enrichedcrystalsis in progress
ZnMoO4 – LUMINEU Aboveground test (CSNSM) of enrichedcrystals 212Pb, 239 214Pb, 295, 352 208Tl, annihil, 511 214Bi, 609 arXiv:1405.6937v1 [physics.ins-det] 228Ac, 911, 969 208Tl, 583 208Tl, 2615
ZnMoO4 – LUMINEU Aboveground test (CSNSM) of enrichedcrystals The enriched crystals behave exactly like the natural ones from any point of view! Muons Light energy [keV] – X-ray calibratedscale 208Tl, 2615 Heatenergy [keV] – gamma-calibratedscale
ZnMoO4 – LUMINEU - Enriched and naturalcrystals in the EDELWEISS cryostat Removing the Cu cover…. Enriched ZMO 1 & 2 Light detector Natural ZMO 1 Natural ZMO 2 …removing the light detector ZMO crystal
LUMINEU and follow-up Phased approach and sensitivity Assuming background at 4 x 10-4 counts / (keV kg y), T=5 y, DE = 6 keV (takingintoaccount 2n pile-up ) EPJC, 72 (2012)1-6 PLB, 710 (2012) 318-323 GEN1 GEN2 This background figure is compatible with the internal contamination alreadymeasured in the ZnMoO4 large mass single modules in the framework of LUMINEU and LUCIFER, especially for the isotope 228Th
LUMINEU and follow-up Phased approach and sensitivity Assuming background at 4 x 10-4 counts / (keV kg y), T=5 y, DE = 6 keV (takingintoaccount 2n pile-up ) EPJC, 72 (2012)1-6 PLB, 710 (2012) 318-323 LUMINEU (in present EDELWEISS) GEN1 Available to LUMINEU GEN2
LUMINEU and follow-up Phased approach and sensitivity Assuming background at 4 x 10-4 counts / (keV kg y), T=5 y, DE = 6 keV (takingintoaccount 2n pile-up ) EPJC, 72 (2012)1-6 PLB, 710 (2012) 318-323 GEN1 GEN2 Available (MoU IN2P3 – ITEP – INFN) Possible use of the EDELWEISS cryostat after EDELWEISS-III 2 year scale Sensitivityat the level of the DBD experiments running or in construction (EXO-200, KamLAND-Zen, GERDA phase 2, CUORE, NEXT)
LUMINEU and follow-up Phased approach and sensitivity Assuming background at 4 x 10-4 counts / (keV kg y), T=5 y, DE = 6 keV (takingintoaccount 2n pile-up ) EPJC, 72 (2012)1-6 PLB, 710 (2012) 318-323 GEN1 GEN2 • Molybdenumcanbeenriched by centrifugation atreasonableprices (50 – 100 $/g) and reasonablethroughput • 350 kg of enriched Mo fits the budget / timescale of a nextgeneration double beta decayexperiment • Novosibirskset-up 8 crystals/monthis possible withonly one furnace
CaMoO4 – AMoRE Crystallization In this case, not onlyenrichment in 100Mo ishighlydesirable, but alsodepleted Ca, withnegligibleamount of 48Ca, isnecessary (background fromtwo neutrino double beta decay of 48Ca, which has Q 4.3 MeV).
CaMoO4 – AMoRE Detector technology In principle, muchbetter S/N ratio than in LUCIFER/LUMINEU Read-out more complicated due to SQUIDs
CaMoO4 – AMoRE Single-module aboveground results M=196 g Excellent technicalresults Veryhigh light yield30,000 ph/MeV(the best among all molybdates) The crystals show a non-negligibleinternal contamination
CaMoO4 – AMoRE Underground installation is in progress
CaMoO4 – AMoRE Phased approach and schedule GEN1 GEN2