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Otto Stern (Sohrau 1888 – Berkeley 1969) Nobel Laureate 1943. Otto Stern, O.R. Frisch, I. Estermann (Hamburg, 1929-1933). He . NaCl(001).
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Otto Stern (Sohrau 1888 – Berkeley 1969) Nobel Laureate 1943
Otto Stern, O.R. Frisch, I. Estermann (Hamburg, 1929-1933) He NaCl(001)
“These experiments are of interest not only because of their confirmation of the predictions of quantum mechanics, but also because they introduce the possibility of applying atom diffraction to investigations of the atomic constitution of surfaces.” (T. M. Johnson, Phys. Rev. 37 (1931) 847).
Bound-state resonances Frisch-Stern (1933) I00 J. E. Lennard-Jones and A. F. Devonshire, Nature 137 (1936) 1069.
Gas – Surface Interactions: - energy transfer - sticking (adsorption) INELASTIC SCATTERING INELASTIC RESONANCES Lattice vibrations (phonons) J.M. Jackson and N.F. Mott, Proc. Roy. Soc. A 137 (1932) 703: Quantum DWBA
L.D. Landau, Phys. Z. Sowjet. 8 (1935) 489. B.L. Bonch-Bruevich, Usp. Fiz. Nauka 40 (1950) 369 Classical Rarified Gas Dynamics Supersonic Molecular Beams
High-resolution diffraction Supersonic He-atom beam sources Time-of-flight spectroscopy
Angular distributions Diffraction Bound state resonances, etc.
Time of Flight (TOF) Inelastic scattering Phonons via the mechanical action (Pauli repulsion) on the electron density Phonon dispersion curves Forces between atoms Forces between ions and electrons (electron-phonon interaction) & electronic susceptibility
Surface waves Lord Rayleigh (1887) Irpinia 1980 (Polo Sismico Alberto Gabriele, FCCSEM Erice)
TOF spectrum Energy-transfer spectrum scan curves for 90° geometry
HAS versus theory NaF(001) LiF(001) theory: Green Function surface dynamics + DWBA scattering theory
HAS hole-electron pairs! 1D conductor electron-hole excitations Peierls instability
The Helium-3 Spin-Echo Spectroscopy P. Fouquet, A.P. Jardine, S. Dworski, G. Alexandrowicz, W. Allison and J. Ellis "Thermal energy 3He spin-echo spectrometer for ultrahigh resolution surface dynamics measurements“ Rev. Sci. Inst. 76, 053109 (2005).
A first test for He3 Spin-Echo: Bound states of He3 on LiF(001) back to Frisch & Stern! A.P. Jardine, S. Dworski, P. Fouquet, G. Alexandrowicz, G.Y.H. Lee, D.J. Riley, J. Ellis, W. Allison, "Ultrahigh resolution spin-echo measurement of surface potential energy landscapes", Science 304, 1790-1793 (2004).
cluster beam cluster assembled film Grenoble - 9 SUPERSONIC CLUSTER BEAM DEPOSITION at the Department of Physics, University of Milano TOF-MS CHAMBER DEPOSITION CHAMBER SOURCE CHAMBER quartz MB sample manipulator He line PMCS substrate time of flight mass spectrometer to pulsed power supply target 2000 l/s diff. pump 700 l/s diff. pump 500 l/s turbo pump
something more in: Giorgio Benedek J. Peter Toennies Helium Atom Scattering Spectroscopy of Surface Phonons Springer-Verlag Berlin Heidelberg New York 2007