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240,242 Pu( n,f ) measurement @ n_TOF. A. Tsinganis (CERN/NTUA) , E. Berthoumieux (CEA Saclay ), M. Calviani (CERN), V. Vlachoudis (CERN). n_TOF Annual Collaboration Meeting Lisbon, December 13-15, 2011. Outline. PART I Samples & detector Samples The Micromegas chamber
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240,242Pu(n,f) measurement @ n_TOF A. Tsinganis (CERN/NTUA), E. Berthoumieux (CEA Saclay), M. Calviani (CERN), V. Vlachoudis (CERN) n_TOF Annual Collaboration Meeting Lisbon, December 13-15, 2011
Outline • PART I • Samples & detector • Samples • The Micromegas chamber • Mounting the samples • Mounting the chamber in the EAR • PART II • Data and analysis • Data • Preliminary analysis • Part III • Simulations • Technique • Results • End goals • Conclusions / To do 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Introduction • An (n,f) measurement on 240,242Pu… • …using a Micromegas detector (FIMG – FIssionMicromeGas) • Proposal CERN-INTC-2010-042 / INTC-P-280 (21/05/2010) • http://cdsweb.cern.ch/record/1266869/files/INTC-P-280.pdf 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Samples • Eight (8) samples (4 x 240Pu, 4 x 242Pu) received from IRMM (Geel) • 3 cm diameter • Chemical form: PuO2(plutonium oxide) • 0.25 mm aluminium backing (5cm diameter) • Mass • ~ 3.5 mg (Pu-240, 99.89%) • ~ 3.0 mg (Pu-242, 99.97%) • Surface density 0.10-0.13 mg/cm2 • Total mass is lower than included in proposal • Activity • 27.3 MBq (Pu-240) • 1.2 MBq (Pu-242) 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
The Micromegas chamber • Designed to hold up to 10 samplesand microbulkMicromegas detectors • …although with some difficulty • BNC connections for signals and HV • Aluminium chamber • Kapton windows • Gas • 88% Ar • 10% CF4 • 2% iso-C4H10 (isobutane) • 1 bar 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Mounting the samples • Mounting carried out in ISOLDE lab under strict RP supervision • Samples placed in appropriate holders for mounting 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Mounting the samples and detectors • Detectors mounted similarly on the internal frame • Finally, the setup looks like this 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Mounting the samples • A 235U sample (for reference) and an empty frame also mounted • Samples and connection arranged as shown Vd2 = 400V 10 9 8 7 6 5 4 3 2 1 Conventional HV supply Vd1 = 400V BEAM CAEN multi-channel HV supply EMPTY Pu-240 Pu-242 U-235 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Mounting the detector in the EAR • FIMG chamber placed downstream of the TAC 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Mounting the detector in the EAR • 16-channel preamplifier • Constructed at INFN-Bari, based on FIC electronics • Electronic protection in place to prevent channel breakage (quite effective, short of 100%) • A second module is available (we have 2 broken channels) • Shielding of pre-amp necessary to reduce γ-flash oscillations • Also HV filters replaced with better shielded ones (provided by E. Griesmeyer) 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Data • Sample signals • Baseline oscillation after γ-flash (down to a few MeV) • Obvious difference in α-activity α FF Pu-242 Pu-240 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Baseline oscillations - grounding • EAR-1 grounding 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Data • Data acquisition in parallel with C6D6 (Ni-58, U-236) and TAC (U-236) measurements • Removed for U-238 TAC measurement • Total protons: • ~ 5 x 1018 (beginning of July – mid-September) • Still short of proposed 8.0 x 1018 • Furthermore, the proposal was based on higher mass and assuming fission collimator setup • Size of data is considerable • Lengthy retrieval, ROOT-file creation and processing times! • Quota issues on lxplus 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Preliminary analysis • The high α-activity of the 240Pu samples makes the pulse recognition routine unworkable in its present form • Routine to be adapted to tackle the problem • The preliminary analysis has thus focused on the 235U reference sample (high counting rate) and 242Pu • The analysis routine for the Diamond detector data (developed by Carlos & Christina) has been used to create the DST files • Retrieval of data very slow due to size of files • ROOT files have been created for only a limited part of acquired data (10% of 2011 statistics) 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Preliminary analysis • Artefacts due to γ-flash oscillations U-235 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Preliminary analysis • Artefacts due to γ-flash oscillations 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Preliminary analysis • Artefacts due to γ-flash oscillations 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Preliminary analysis • Amplitude spectrum – alpha/FF separation U-235 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Preliminary analysis • U-235 resonances 1-10eV • Compared with ENDF VII
Preliminary analysis • Pu-242 at threshold • Compared with ENDF VII ~10% of 2011 statistics 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations • FLUKA simulations • Attempt to reproduce signals from α-particles and fission fragments • α-particles and fission fragments studied separately • Initial position sampled randomly within the sample volume • Particles emitted isotropically within 2π solid angle • Alpha-particles • Energy: 5.2MeV • Fission fragments • Mass and energy systematics from G.D.Adeev et al., Preprint INR 861/93 1993 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations • Simplified geometry created in FLUKA • Simulation of samples and active detector volume • Energy deposition along z-axis is scored event-by-event • From energy deposition to charge (~26eV / electron-ion pair) Gas Sample dE/dz 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations • Electron drift velocity calculated for given gas mixture and drift voltage • …using GARFIELD 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations • Simplified geometry created in FLUKA • Simulation of samples and active detector volume • Energy deposition along z-axis is scored event-by-event • From energy deposition to charge (~26eV / electron-ion pair) • Electron drift velocity calculated for given gas mixture and drift voltage • …using GARFIELD • …we can thus calculate the current reaching the readout electrode • This signal is passed through a CR-RC circuit to obtain the final pulse • Typical amplifiers use a CR-(RC)4 circuit to achieve a quasi-gaussian pulse shape Gas V Sample dE/dz 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations: data reconstruction • A large time window is selected in which we randomly add: • White noise • α-particle and fission fragment pulses • …at appropriate rates 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations: data reconstruction • Total (mixed) signal: 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations: data reconstruction • Each component is known… 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Simulations: data reconstruction • …we can therefore apply the pulse recognition routine used for the experimental data and attempt to reconstruct an amplitude spectrum Counts α-particles The quality of the α – FF separation can then be estimated Amplitude cut Fission fragments Noise Amplitude 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
Conclusions • To do: • Fix analysis routine to address: • γ-flash oscillation • α-activity in 240Pu • Carry on with data processing and analysis (obviously) • Finalise simulations • Create realistic signals for different count rates • Pulse recognition routine • Study α – FF separation • Compare with experimental amplitude spectrum • Study pile-up probability • Detector efficiency • Once simulations are in place, the same technique can be used for the fission tagging measurements • FIMG chamber with Pu samples presently stored by RP in view of the 2012 run • Accumulate as much statistics as possible within 2012 planning • Actions during winter shutdown • Address grounding issues in EAR-1 (general action) • Investigate shielding improvement of pre-amp box 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.
The end 240,242Pu(n,f) measurement @ n_TOF n_TOF Annual Collaboration Meeting – Lisbon, December 13-15, 2011 | A.T.