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Nuclear Fission. Liquid-Drop Oscillations. Bohr&Mottelson II, Ch. 6. Surface & Coulomb energies important: Stability limit C l 0. Fissility. Mostly considered: small quadrupole and hexadecapole deformations b 2 =a 20 ≠0 ≠ b 4 = a 40 But b 3 = 0 (odd electrostatic moment forbidden).
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Nuclear Fission Spontaneous Fission
Liquid-Drop Oscillations Bohr&Mottelson II, Ch. 6 Spontaneous Fission Surface & Coulomb energies important: Stability limit Cl 0
Fissility Mostly considered: small quadrupole and hexadecapole deformations b2=a20≠0 ≠ b4=a40 But b3=0 (odd electrostatic moment forbidden) Bohr-Wheeler fissility parameter Stability if x < 1 Spontaneous Fission
b4 PES b2 Cut along fission path Fission Potential Energy Surface Fission path Q Saddle CN Spontaneous Fission mCNc2 FF1 FF2 2mFc2 Typical fission process:
LDM-Fission Saddle Shapes Spontaneous Fission Cohen & Swiatecki, 1974
Systematics of Fission Total Kinetic Energies Viola, Kwiatkowski & Walker, PRC31, 1550 (1985) Average total kinetic energy <EK>of both fission fragments as function of fissioning compound nucleus (CN) Z and A: Spontaneous Fission
FF1 FF2 r Viscosity in Fission For high fissilities (elongated scission shapes) kinetic energies smaller than calculated from saddle Coulomb repulsion: TKE < Tf (∞) viscous energy dissipation. Nix/Swiatecki : Wall and window formula (nucleon transfer, wall motion) Spontaneous Fission Viscosity 25% of strength in HI collisions Davies et al. PRC13, 2385 (1976)
P(b,t) time b V(b) saddle point Kramers’ Stochastic Fission Model Grange & Weidenmüller, 1986 Collective d.o.f. (b) coupled weakly to internal (nucleonic) d.o.f. ttrans Spontaneous Fission b Gradual spreading of probability distribution over barrier (saddle). Probability current from jF =0 to stationary value at t ∞
V(b) Inverted parabolaOscill frequ. wsad Fission Transient and Delay Times Statistical Model fission life time: Level Density Spontaneous Fission Concepts revisited by H. Hofmann, 2005/2006
Prescission Neutron Emission D. Hinde et al., PRC45, 1229 (1992) Exptl. setup detects FF, lcps, and n in coincidence decompose angular distributions Sources CN, FF1, FF2 Spontaneous Fission Short fission times for high E*> 300-500 MeV ? Systematics: WUS et al. Berlin Fission Conf. 1988
Pre-neutron emission Post-neutron emissionRadio-chemical data 232Th(p, f) Ep = yield nn(A) nn(A) FF Mass A Fission Fragment Mass Distributions E* Dependence of FF Mass Distribution: asymm symm nn(A) Spontaneous Fission H. Schmitt et al., PR 141, 1146 (1966) Neutron emission in fission: n ≈ 2.5±0.1 Croall et al., NPA 125, 402 (1969)
yield <Alight> <Aheavy> ACN Fission Fragment Z Distributions Vandenbosch & Huizenga, 1973 Bimodal mass distributions: With increasing ACN more symmetric. <Aheavy> ≈ 139 shell stabilized via <Zheavy>≈ 50 Spontaneous Fission Zp: The most probable Z Same Gaussian A(Z-Zp)
Rsc Z P(Z) V Models for Isobaric Charge Distributions Unchanged charge distribution (UCD): Experimentally not observed, but Minimum Potential Energy (MPE) Models Spontaneous Fission App. correct for asymmetric fission (DZ ≈ +0.5).Incorrect: o-e effects, trends DZ ≈ -0.5 at symmetry. MPE variance: expand V around Z=Zp:
Rsc A Z V(Z,N) P(Z,N) A=const. N Models for Isobaric Charge Distributions Try thermal equilibrium (T): Linear increase of s2 with T not observed, but s≈ const. up to E*<50MeV Spontaneous Fission dynamics? NEM ? Studied in heavy-ion reactions.
TKE TKE Mass-Energy Correlations Pleasanton et al., PR174, 1500 (1968) asymmetric fission: p conservation 235U +nth Fission Energies 235U +nth EF1-EF2 Correlation FF mass ratio Spontaneous Fission heavy light Pulse heights in detectors affected by pulse height defect
match to incoming wave Fine Structure in Fission Excitation Functions I II Spontaneous Fission J. Blons et al., NPA 477, 231 (1988) Also: g and n decay from II class states Class I and II vibrational states coupled
Shell Effects in Fission LDM barrier only approximate, failed to account for fission isomers, structure details of sf. Shell effects for deformation Nilsson s.p. levels accuracy problem Strutinsky Shell Corr. Spontaneous Fission In some cases: more than 2 minima, different 1., 2., 3. barriers
Angular Distribution of Symmetry Axis Spontaneous Fission