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Nuclear effects in the optically-detected magnetic resonance of electron spins in n-GaAs

This study delves into the impact of nuclear effects on optically-detected magnetic resonance of electron spins in n-GaAs. The research covers Overhauser Coupling, quantum well samples, resonance conditions, and the Modified ODENDOR method. Results reveal insights into nuclear polarization changes, spin oscillations, and DNP control. The comparison between bulk and Quantum Well samples underscores the varying sensitivities and coupling strengths. The study highlights the significance of monitoring resonating nuclei and controlling DNP within certain limits. The research team expresses gratitude to John Colton, Brigham Young University, and other contributors for valuable insights and support.

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Nuclear effects in the optically-detected magnetic resonance of electron spins in n-GaAs

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  1. Benjamin Heaton John Colton Brigham Young University Nuclear effects in the optically-detected magnetic resonance of electron spins in n-GaAs

  2. Outline 1) Background 2) Overhauser Coupling and DNP 3) Control of Nuclear Effects 4) Modified ODENDOR Method and Results 5) Quantum well sample 6) Oscillations in spin polarization

  3. Increasing Average μ-wave Power Resonance Conditions Nuclear polarization changes Electron polarization changes Increasing ESR μ-wave Power Increasing Laser Power Overhauser effect causes broadening and shifting of the ODMR peak “Bulk” = 3E14 n-GaAs “QW” = 3e12, 14nm well

  4. Time Time Nuclear relaxation time Nuclear spin has a lifetime of 2.3 minutes

  5. NMR coils Split Helmholtz coil creates oscillating magnetic field at NMR frequencies Resonated nuclei have zero net polarization DNP is eliminated Take off numbers

  6. 75As Nuclei Modified ODENDOR on two Ga isoptopes and 75As Although no new information is gained through this process, this new method of measuring nuclear spin resonance is shown to be viable. More importantly, we have complete control over DNP! • 1) Resonate two of the three nuclei • 2) Monitoring ODMR peak • 3) Stepping through the third nuclei. Nuclear resonance peak is very narrow! 10KHz and pushing the limits of our sensitivity

  7. Not really “complete” control:(two competing effects)‏ DNP vs. Resonating field of our Helmholtz coil B = (n*I)/R Good News: Quantum well sample has less Overhauser coupling.

  8. Sensitivity to wavelength Similar samples have been studied with pulsed lasers. Our CW laser has narrow enough bandwidth to see wavelength dependence This frequency dependence was not seen in the bulk GaAs sample

  9. Microwaves turn on Microwaves turn on Long T1≈ 50 μs Short T1≈ 200ns Spin Oscillations Quantum Well Sample Bulk Sample

  10. Probably not Rabi flopping:Definitely due to oscillations in spin polarization • Turns on and off with the electron spin resonance conditions • Oscillations present at 1.5K, but not at 5K • Doesn't have the correct dependence on field to be coherent precession • Doesn't have the correct dependence on ESR power to be Rabi oscillations

  11. Conclusion • We can control the DNP (within certain limits)‏ • Modified ODENDOR method works • We see unexplained spin state oscillations • Compare QW and bulk GaAs samples • Bulk Sample • Strong Overhauser Coupling • Insensitive to probe wavelength • Long T1 • T2* = 20 ns • Quantum Well Sample • Weak Overhauser Coupling • Very sensitive to probe wavelength • Short T1 • T2* = 6 ns Thanks to: John Colton and his lab group, Mitch Jones, Steve Brown, Michael Scott Tom Kennedy, NRL for useful discussions Berry Jonkers, NRL for the samples NSF for funding

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