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Cavity Solitons : the semiconductor experimentalist's point of view. Robert Kuszelewicz. Laboratoire de Photonique et de Nanostructures LPN-CNRS/UPR20, Marcoussis, France. What is at stake ?. Cavity solitons have a double concern : Fundamental :
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Cavity Solitons : the semiconductor experimentalist'spoint of view Robert Kuszelewicz Laboratoire de Photonique et de Nanostructures LPN-CNRS/UPR20, Marcoussis, France
What is at stake ? • Cavity solitons have a double concern : • Fundamental : • Phenomena, concepts and theoretical approaches of non linear pattern formation • Applied : Original Functions, all-optical signal processing. III-V Semiconductor materials are at the crossroad of two streams of interest. • Strong intensity-dependent nonlinear optical properties near the band gap edge • Integrability and ability to realise a large variety of optical devices with a complete crystal compatibility (compacity)
Purpose of the lecture • Show how theoretical concepts pertaining to TNO can be implemented into physical systems • Draw a short history of the most striking advances with various materials : • Na-vapor, LCLV, III-V semiconductors • Concentrate on semiconductor systems : • State of the art • Advantages, limitations, drawbacks • Capabilities and expectations
Outlines • Materials : • Na-vapour, LCLV and III-V semiconductors Mechanisms for Transverse Nonlinear Optics: • Nonlinearity • Competition mechanisms • Transverse mechanisms Phenomena : • From bistability to spatial pattern formation ... Transverse Nonlinear Optics Description of various systems : • Passively injected systems • Amplifying injected systems • Laser systems : injected or saturable absorber Limitations : • Uniformity : thickness, current, defects • Thermal effects : Production, dependance and dissipation What to do with ? • Functions, processing
Material systems and related optical models Liquid Crystal Light Valves Kerr-like dispersive medium Sodium Vapor : Two-level system : saturable dielectric function III-V semiconductors Electronic bands : Dynamical response Many-body interactions Dielectric function
LCLV : the Pure Kerr-model Residori et al., J. Opt. B: Quantum Semiclass. Opt. 6 (2004) S169–S176
The two level system : optical response • Positive or negative nonlinear dispersion • Inversion of properties above transparency
The bulk semiconductor model Direct gap semiconductors Parabolic model + Exciton Many-body effects + Band filling + Coulomb interactions Electron screening, Band gap renormalisation Exchange interaction
Recombination mechanisms Radiative Stimulated Spontaneous Auger phonon-assisted Non radiative Recombinations on defects Electron-phonon Direct Indirect
Dynamical regimes • Characteristic timescales Dephasing time Time after which phase relation is lost between the polarisation and the exciting field Populations lifetime Relaxation time of excited populations (probabilities) In general For III-V materials , Excitation duration • Dynamical regimes : ultra short pulses. Coherent transients : photons écho, superradiance, self-induced transparency.. Dynamical Stark Effect : : Dynamic nonlinearities. Polarization quasi-steady state vs Electric field. NL response ruled by the evolution of excited populations : intraband relaxation : quasi-stationnary situation : adiabatic elimination of the carriers
Carrier dynamics Excitation of optically coupled states Intraband dynamics of carriers
The direct gap semiconductor dielectric function The Carrier density-dependant susceptibility with and without many-body effects (Koch model) Real and imaginary part are connected by the Kramers-Kronig transform : -factor derives as so that
QD susceptibility InAlAs/GaAlAs QD Density ~ 1011 cm-3 Inhomogeneous broadening Inhomogeneously broadened optical response Dynamic model of QD
Observations • The properties of the susceptibility in III-V semiconductor are multifactorial : • High background index n~3.5, • Strong NL in the vivinity of the band gap, • In the passive case, the NL dispersion is defocusing • Above transparency, focusing NL appear • III-V semiconductor are highly temperature-sensitive • via the shift of the band gap • Quantum dots seem quite a promising alternative for focusing NL
Mechanisms of TNO • Transverse Nonlinear Optical phenomenarequire : • Kerr-like or saturable intensity-dependent susceptibility • Positive feedback : Fabry-Perot resonance or feedback mirror enforces light-matter interaction duration yielding a “catastrophy”. Mechanism with threshold : NL + feedback PW bistability • Transverse effects : diffraction, diffusion Create the conditions of non locality. Mechanism with threshold : MI The conjunction of these three mechanisms generate the spatio-temporal dynamics.
Phenomena From bistability to spatial pattern formation ... Transverse Nonlinear Optics • PW bistability : thermal / electronic NL • Switching waves BISTABILITY + LARGE FRESNEL NUMBER • Pattern formation • Localised states
Devices • Description of various classes : • Passive injected systems : Na vapours and III-V semiconductors • Injected amplifying systems : optically- and electrically- pumped VCSEL • Laser systems : injected or saturable absorber systems
Na-vapor feedback mirror systems (Muenster univ.) • Drift in a gradient • Modulated landscape
LCLV in a feedback loop Patterns and localised states Non local interactions
Semiconductor systems Experimental system (LPN, PTB)
Switching waves Outward front Maxwell point Inward front
Injected semiconductor amplifiers • Arguments on the interest for over transparency operation • Positive : dispersive confinement • Amplification : cascadability • Two similar approaches : • Electrical pumping • INLN • Optical pumping • LPN • Discussion on the respective interest of each
Pump I Electrical vs Optical pumping
L = 1 Ûtransparency L = 1+1/2C Ûlaser threshold C largesmall excursion range in terms ofL smalla C small large excursion range in terms of L large a Theoretical model for field and carriers C : bistability parameter L : pump a : Henry factor [M. Brambilla, L. Lugiato, F. Prati, L. Spinelli, W. Firth, PRL 79, 2042 (1997)] Good compromise : C ≈ 0.5 high finesse cavity
Electrically injected VCSELs Bottom emitting laser (ULM)
The initial demonstration : independance of 2CS Writing Erasure sequence of 2 CS (Barland et al., Nature 419, 699(2002)
Interplay with non uniformity The thickness gradient scans the state space through the detuning parameter 80 mm Seven CS
Optical pump fewer technological steps, less heating Absorbing spacers Active layer Front mirror Aperiodic back mirror Pump window Cavity resonance Cavity design for optical pumping [Y. Ménesguen, R. Kuszelewicz, to appear IEEE-JQE 41,N°7 (2005)] [S. Barbay, Y. Ménesguen, I. Sagnes, R. Kuszelewicz, APL 86, 151119 (2005)]
Experimental setup Large-area semiconductor amplifier in AlGaAs/GaAs
Decreasing l 888.62 nm 890.98 nm 889.95 nm 889.27 nm 888.23 nm Results / pattern formation
Pump + injection 888.38nm 120 mm Increasing Pumping Spontaneous formation of CS Pump
Independance and multiplicity of CSs Independence of 2 CS W/E in the vicinity of 3 other CS Y. Ménesguen, S. Barbay, X. Hachair, L. Leroy, I. Sagnes and R. Kuszelewicz, submitted PRA (2006)
Hysteresis Local reflected intensity HB power Field Carriers
CS on ~5 ns CS on ~2ns 60 ps writing pulse CS off CS off Fast incoherent writing/erasure : 60ps pulses Repeated writing and reset writing erasure
Laser systems Optically pumped monolithic active cavity with SA • Why going above threshold ? • Cascadability • Diversification of the bistable mechanisms • Injection or feedback lasers : mode competition • Saturable absorber (SA): gain loss competition • With SA, no holding beam is necessary • Incoherent switching
Feedback laser Bistable localised states(Y. Tanguy, T. Ackemann, USTRAT) 80mm Laser (ULM) spatially filtered feedback,appear spontaneously at preferential locations Frequency tuning dependence With 200 mm, LS can be written without spatial filtering
QW gain medium(/QD?) Laser field Pump field QW or QD saturable absorber Saturable Absorber Semiconductor lasers (LPN) Optically pumped monolithic active cavity with SA OP-VCSELSA • Need a cavity with special requirements • Very good cavity finesse around lasing wavelength (use QW) • pump window (OP) + optimized pumping • Saturable absorber section • no pump field but laser field • Gain section • pump field & laser field
Front mirror Back mirror Laser field ~980 nm Pump fields 795-805 nm SA section Gain section 1 InGaAs/AlGaAs QW 2 InAs/GaAs QW OP-VCSELSA cavity design Experiment :Optically pumped monolithic active cavity with SA Theory :Laser with SA (coll. INFM/Como) QD model (coll. INFM/Bari) Simplex optimization procedure on layer thicknesses : front and back mirror R,T front and back mirror jR, jT overall cavity A