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National/Regional Air Quality Modeling Assessment Over China and Taiwan Using Models-3/CMAQ Modeling System. Joshua S. Fu 1 , Carey Jang 2 , David Streets 3 , Zuopan Li 1 , Litao Wang 4 , Qiang Zhang 4 , Binyu Wang 2 , Jung-Hun Woo 5 , Der-Ming Tsai 6 and Yu-Lin Wu 6
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National/Regional Air Quality Modeling Assessment Over China and Taiwan Using Models-3/CMAQ Modeling System Joshua S. Fu1, Carey Jang2, David Streets3, Zuopan Li1, Litao Wang4, Qiang Zhang4, Binyu Wang2, Jung-Hun Woo5, Der-Ming Tsai6 and Yu-Lin Wu6 1University of Tennessee, USA 2U.S. Environmental Protection Agency, USA 3Argonne National Laboratory, USA4Tsinghua University, China 5University of Iowa, USA 6National Chen Kung University RTP, NC, October 20, 2004
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Models-3/CMAQ Study Domains Domain : Great China Region Grid Resolution : 36-/12-/4-km (Nested Modeling) Episode : July 1-20, 2001 January 1-20 , 2001
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 China National/Regional Modeling Configuration • Features : Models-3/CMAQ One-Atmosphere (multi-pollutants) Run • July and January 2001 CMAQ Runs • Nationwide, East China/Beijing CMAQ Domains • Model Setup : • NASA’s TRACE-P emission inventories and Beijing local emissions and GEIA biogenic emission inventory • Emissions Processing: Spatial allocation (GIS/Gridding), Temporal, speciation needed for the M3/CMAQ simulations • 36-km (164x97), 12-km (175x211), and 4-km (160x142), (90x90), (97x133), 14 vertical layers • Meteorology : MM5 V3.6.2 • CMAQ (February, 2004 version)
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 China National/Regional Application Ozone • Layer distribution : • Layer 1: 38 m • Layer 2: 91.5 m • Layer 3: 152.9 m • Layer 4: 230.3 m • Layer 5: 339.5 m • Layer 6: 481.6 m • Layer 7: 845.8 m • Layer 8:1300.7 m • : • : • Layer 14: 16262.4 m
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Convert TRACE-P emission data to CB IV Speciations
------------------------------------------------------------------------------------ Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 China Regional Modeling (Nesting): O3 36-km 12-km 4-km
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 NOx Emissions (36kmx36km) TRACE-P January EM TRACE-P July EM
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 NOx Emissions (12kmx12km) TRACE-P January EM TRACE-P July EM
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 NOx Emissions (4kmx4km) TRACE-P January EM TRACE-P July EM
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 NOx Emissions (4kmx4km) Beijing EMISSION TRACE-P EMISSION
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 SO2 Emissions (4kmx4km) Beijing EMISSION TRACE-P EMISSION
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 PAR Emissions Beijing EMISSION TRACE-P EMISSION
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Difference of PAR Emissions Beijing EMISSION – TRACE-P EMISSION
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Wind Field
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 China Regional Modeling (Nesting): O3 36-km 12-km 4-km (2PM July 15 , 2001.)
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Air Quality Modeling Assessment in Beijing (base case- July 2001) Ozone TRACE-P EMs Beijing EMs
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Beijing Regional (4-km) Modeling: O3 TRACE-P EMs Beijing EMs (July 4-20, 2001, episode max.)
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Sensitivity runs for Beijing region (base case- July 2001) Ozone Beijing EMs 2xVOC Beijing EMs 3xVOC Beijing EMs
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Sensitivity runs for Beijing region (base case- July 2001) Ozone Beijing EMs 2xVOC Beijing EMs 3xVOC Beijing EMs (July 4-20, 2001, episode max.)
Episodic Max O3 (2001 July ) Transported No transported Zero out
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 O3 Daily Max (2001 July )
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Beijing Regional (4-km) Modeling: PM 2.5 January July 75 ug/m3 150 ug/m3 (Jan./July 4-20, 2001, episode avg.)
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 PM2.5 Composition in Beijing (Jan.) M3/CMAQ (4-km) January 4-20, 2001 PM2.5: 154(ug/m3 ) PM2.5 Composition in Beijing (July) M3/CMAQ (4-km) July 4-20, 2001 PM2.5: 99(ug/m3 )
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Episodic AVG PM2.5 (2001 July ) Nested BC Background BC Zero out
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 cn4B0 PM 2.5 Daily MAX Animation (2001 July )
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 CMAQ vs. Obs. PM 2.5 Episode Average 154 140 99 88
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Models-3/CMAQ Pilot Study Domains Domain : Greater China Region Grid Resolution : 36-km/12-km/4km (Nested Modeling) Episodes : Jan. (Jan., April, Oct.) , 2001
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Taiwan Regional Air Quality ModelingPreliminary Results for January Case • Features : • Models-3/CMAQ One-Atmosphere (multi-pollutants) Run • Model Setup : • NASA’s TRACE-P emission inventories and GEIA biogenic emission inventory and TEDS • Emissions Processing: Spatial allocation (GIS/Gridding), Temporal, speciation and SMOKE needed for the M3/CMAQ simulations • Domains: 36-km (130X94),12-km (135X198) and 4-km (56X108), 12 vertical layers • Meteorology : MM5 (V3.5) considered snow cover, NCEP data for IC and BC • CMAQ 4.3
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Air Quality Modeling over China & Taiwan :Model Nesting 12-km 4-km 36-km
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Wind Field
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 The Effects of Air Pollutants Transport in Taiwan Ozone Background air BC Nested air BC Diff
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Nested Modeling at Different Grid Resolution: PM 2.5 4-km (non-nested) 12-km 36-km Taiwan (Jan. 4-20, 2001, episode avg.)
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 The Effects of Air Pollutants Transport in Taiwan PM2.5 Background air BC Nested air BC Diff
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 The Effects of Air Pollutants Transport in Taiwan Visibility (Deciview) Background air BC Nested air BC Diff
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Summary • The first ever application using “One Atmosphere” CMAQ modeling system for Beijing regional air quality modeling • Emissions: Investigate Trace-P Asian emissions and apply Beijing local emissions and Taiwan emission inventory, especially NOx, SO2 and VOC emissions, e.g., ALD2, OLE, PAR. • The use of monitoring data is essential to against CMAQ modeling results • CMAQ model performance is acceptable for PM25 but ozone concentrations are under predicted • VOC found that it may be underestimated in China from sensitivity runs
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Summary • Models-3/CMAQ has been tested for January and July scenarios in national/regional/urban scales in China and Taiwan • 36-km, 12-km and 4-km. • Select typical episodes in January, and October-November (O3), 2001 to further study for the China and Taiwan 4-km domains.
------------------------------------------------------------------------------------- Models-3/CMAQ Workshop, RTP, NC, October 20, 2004 Acknowledgment • USEPA and Taiwan EPA funding support • University of Tennessee Office of Research • Argonne National Laboratory • Tsinghua University • University of Iowa • National Cheng Kung University